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I'd be inclined to think that two non-matching cards is likely to cause you significant grief, to the point that three monitors on the 750 may be more successful than two on the 750 and one on another card.
You might see an improvement in other games, if you use the 640 for PhysX processing. However, it's so much slower than the 750 Ti that even then it might actually make things worse rather than better.