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Flats are most strongly associated with Jazz tones. They are also popular with some slide players who wish to reduce the noises that roundwounds can produce.
I have only ever used flats on fully hollow body electric guitars and, of course, bass.
Very much an acquired taste - I prefer the D'addario 1/2 wound which is effectively a hy-brid of flat and wire wound
Generally the tension of a set of flats is lower on the wound strings because the core of the string under the wrap is smaller, so for most manufacturers, it’s best to assume that the next gauge “up” is relative - basically, if you play a 10-46 gauge roundwound set, go 11-48 or whatever for flats. Thomastik’s have the lightest tension of all flat manufacturers in my experience, so be more aware of this if you try one of their sets.
If you search online you will no doubt come across LaBella Nylon Tapewound strings. These are great on an archtop but go for the 14 gauge set if you’re going to try them. The low strings are very thick so expect some nut, tuning post and maybe even tailpiece adjustments depending on what guitar you have
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Wouldn't it sound weird to have the bottom 3 strings sounding so different?
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Might be different with the much thinner strings on guitar but on bass, roundwounds are quite similar to guitar strings (both roundwound and plain) in that they're bright and have sustain but flatwounds are dull and thumpy - a great sound in its own right, I just think it might be weird going between one and the other.
Maybe they're used mostly for chords where it's always a combination of the two? Or maybe the player always takes the differences in to consideration and only goes to the specific strings when wanting a specific tone?
Edit: for interest sake, he uses a heavy set, drops the low E (old A string is the new E etc)and adds a high E.
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